2024
DOI: 10.1021/acsmaterialslett.4c01150
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Building Stable Pillar-Layered Metal–Organic Frameworks: Introduction of Unsaturated Bonds for Enhanced Efficiency in C2H2/CO2 Separation

Wenke Yuan,
Panyue Guo,
Weize Wang
et al.

Abstract: Pillar-layered structures represent a significant category within MOFs; however, the exploration of their chemical stability and systematic functionalization has been largely neglected. Herein, we fabricated a pillarlayered MOF (Zn-L C−C ) with fsc topology, utilizing a tetradentate carboxylic ligand with bipyridine and Zn(II) ions via the pillar-layered approach. Notably, this topological structure displays markedly superior stability compared with typical pillar-layered MOFs with pcu topology. In addition, b… Show more

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