Squeak and rattle belong to unintended noise audible by occupants of a vehicle. This noise negatively affects the perceived built quality, leading to nonbuying decisions, high warranty costs, and poor brand reputation. Therefore, vehicle manufacturers seek to prevent the emergence of such noise, preferably in the early development phase and during production at the latest. This causes substantial monetary and temporal expenditure, which must be minimized. Rattle is defined as repeated impact. The underlying physical phenomenon is impulsive short‐duration contact normal to the surface. Squeak, in contrast, originates from an in‐contact motion in the tangential direction and is a friction‐induced stick‐slip phenomenon. State‐of‐the‐art numerical squeak and rattle prediction is based on linear analysis resulting in an empirical noise risk index. However, quantification of noise and assessment of audibility is not possible. The reason is the nonlinearity of the contact forces. Hence, the actual system response is not calculable with a linear approach. Mathematically, the nature of both excitation events is nonlinear due to frictional contact and nonsmooth due to short impulsive behavior in time. This makes linear simplification and a solution process in the time domain challenging. Both events appear periodically, leading to an oscillation characterized by fundamental and higher harmonics. Due to this periodic character, squeak and rattle phenomena fulfill the prerequisite for applying the harmonic balance method (HBM) to solve the governing nonlinear equation of motion. The more harmonics considered, the more precise the modeling and the dynamic response prediction. In addition, the alternating frequency/time domain method (AFT) allows for switching between the frequency and the time domain during the iterative solution process. Thus, the nonlinear contact forces can be evaluated in the time domain. The equation‐solving process results in the calculation of surface velocities. This gives way to determining a proxy for the emitted sound power of the oscillatory system. The simulation method based on combining HBM and AFT was validated on test rigs for squeak and rattle noise. The industrial applicability of this simulation approach was demonstrated numerically and experimentally on an actual vehicle part showing promising results. Thereby, important steps in nonlinear structural dynamics and vehicle acoustics were made toward a calm, smooth, and enjoyable ride for vehicle occupants.