The present research work describes the fabrication and interlaminar properties testing of carbon fiber aluminum metal laminates (CARALL). CARALL was fabricated through hand layup process followed by compression molding technique and interlaminar properties were assessed through double cantilever beam (DCB) test short beam and flexural test. Different treatments were performed on the surface of aluminum alloy and parameters were optimized to ensure good adhesion between metal sheet and carbon composite layer. Pull-off adhesion test was performed to gauge the adhesion strength of epoxy resin on aluminum alloy sheet. Effect of Multi-wall carbon nanotubes (MWCNTs) was also investigated on the interlaminar properties of CARALL. Treated surface of aluminum alloy sheet was examined under Optical and Field Emission Scanning Electron Microscopy (FE-SEM). Porous surface was evident on aluminum sample due to surface treatment which contributes towards better adhesion between epoxy resin and metal surface through mechanical interlocking and diffusion mechanism. FE-SEM and stereo microscopy was also performed on fractured DCB samples and underlying fracture mechanism was discussed. Test results demonstrated that addition of MWCNTs deteriorated the interlaminar properties of CARALL by weakening the interface between treated aluminum surface and carbon composite.