Carbon Capture and Storage in Geologic Formations

Ussiri, David A.N.; Lal, Rattan

doi:10.1007/978-3-319-53845-7_13

Carbon Sequestration for Climate Change Mitigation and Adaptation 2017

DOI: 10.1007/978-3-319-53845-7_13

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Carbon Capture and Storage in Geologic Formations

David A.N. Ussiri

Rattan Lal

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Cited by 3 publications

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Through‐Space Electrostatic Interactions Surpass Classical Through‐Bond Electronic Effects in Enhancing CO₂ Reduction Performance of Iron Porphyrins

et al. 2021

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In his pioneering work to unravel the catalytic power of enzymes, Warshel has pertinently validated that electrostatic interactions play a major role in the activation of substrates. Implementing such chemical artifice in molecular catalysts may help improve their catalytic properties. In this study, a series of tetra‐, di‐, and mono‐substituted iron porphyrins with cationic imidazolium groups were designed. Their presence in the second coordination sphere helped stabilize the [Fe−CO2] intermediate through electrostatic interactions. It was found herein that the electrocatalytic overpotential is a function of the number of embarked imidazolium. Importantly, a gain of six orders of magnitude in turnover frequencies was observed going from a tetra‐ to a mono‐substituted catalyst. Furthermore, the comparative study showed that catalytic performances trend of through‐space electrostatic interaction, a first topological effect reported for iron porphyrins, outperforms the classical through‐structure electronic effect.

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Through‐Space Electrostatic Interactions Surpass Classical Through‐Bond Electronic Effects in Enhancing CO₂ Reduction Performance of Iron Porphyrins

et al. 2021

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Environmental and safety issues associated with geological carbon storage: a review

Chijioke

Opara

Onyekuru

et al. 2022

Euro-Mediterr J Environ Integr

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Governance of bioenergy with carbon capture and storage (BECCS): accounting, rewarding, and the Paris agreement

Torvanger

2018

Climate Policy

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Carbon Capture and Storage in Geologic Formations

Cited by 3 publications

References 115 publications

Through‐Space Electrostatic Interactions Surpass Classical Through‐Bond Electronic Effects in Enhancing CO₂ Reduction Performance of Iron Porphyrins

Through‐Space Electrostatic Interactions Surpass Classical Through‐Bond Electronic Effects in Enhancing CO₂ Reduction Performance of Iron Porphyrins

Environmental and safety issues associated with geological carbon storage: a review

Governance of bioenergy with carbon capture and storage (BECCS): accounting, rewarding, and the Paris agreement

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Carbon Capture and Storage in Geologic Formations

Cited by 3 publications

References 115 publications

Through‐Space Electrostatic Interactions Surpass Classical Through‐Bond Electronic Effects in Enhancing CO2 Reduction Performance of Iron Porphyrins

Through‐Space Electrostatic Interactions Surpass Classical Through‐Bond Electronic Effects in Enhancing CO2 Reduction Performance of Iron Porphyrins

Environmental and safety issues associated with geological carbon storage: a review

Governance of bioenergy with carbon capture and storage (BECCS): accounting, rewarding, and the Paris agreement

Contact Info

Product

Resources

About

Through‐Space Electrostatic Interactions Surpass Classical Through‐Bond Electronic Effects in Enhancing CO₂ Reduction Performance of Iron Porphyrins

Through‐Space Electrostatic Interactions Surpass Classical Through‐Bond Electronic Effects in Enhancing CO₂ Reduction Performance of Iron Porphyrins