Carbon layer confined Co–Ni bimetallic oxide heterojunctions for high-efficiency electrosynthesis of 2,5-furandicarboxylic acid

Cheng, Zhong; Hu, Jing; Zhou, Wenjing; Deng, Wenfang; Ma, Ming; Tan, Yueming

doi:10.1039/d4ta01159g

J. Mater. Chem. A

2024

DOI: 10.1039/d4ta01159g

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Carbon layer confined Co–Ni bimetallic oxide heterojunctions for high-efficiency electrosynthesis of 2,5-furandicarboxylic acid

Zhong Cheng,

Jing Hu,

Wenjing Zhou

et al.

Abstract: Electrooxidation of 5-hydroxymethylfurfural (HMF) has been recognized as an efficient method for obtaining high value-added chemicals, so it is desirable to develop highly active and stable catalysts for electrocatalytic HMF...

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Stabilizing Ni³⁺ Species through High-Valence Molybdenum Introduction for 5-Hydroxymethylfurfural Electrooxidation

Zhang,

Xiao,

et al. 2024

Ind. Eng. Chem. Res.

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5-Hydroxymethylfurfural (HMF) electrooxidation for 2,5-furandicarboxylic acid (FDCA) production has become a sustainable method for value-added products at the anode. Here, an amorphous NiMo composite oxide supported on nickel foam (NF) is fabricated for HMF electrooxidation (HMFOR) via one-step electrodeposition. The synthesized NiMo/NF delivers 98.3% FE toward FDCA at 1.5 V RHE and maintains FE above 90% during 10 h. In situ Raman spectroscopy proves the formation of the active species Ni 3+ -OOH during the reaction process. Due to the introduction of high-valent Mo 6+ , the Ni 3+ active species can be stabilized and the adsorption of aldehyde in HMF can be promoted during the reaction process, thus enhancing the FDCA electrosynthesis performance.

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Stabilizing Ni³⁺ Species through High-Valence Molybdenum Introduction for 5-Hydroxymethylfurfural Electrooxidation

Zhang,

Xiao,

et al. 2024

Ind. Eng. Chem. Res.

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Electrochemical glucose-to-formic acid conversion coupled with alkaline hydrogen production over nanostructured CuCo₂O₄ catalysts

Lin,

Xue,

2024

J. Mater. Chem. A

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Carbon layer confined Co–Ni bimetallic oxide heterojunctions for high-efficiency electrosynthesis of 2,5-furandicarboxylic acid

Abstract: Electrooxidation of 5-hydroxymethylfurfural (HMF) has been recognized as an efficient method for obtaining high value-added chemicals, so it is desirable to develop highly active and stable catalysts for electrocatalytic HMF...

Cited by 2 publications

References 43 publications

Stabilizing Ni³⁺ Species through High-Valence Molybdenum Introduction for 5-Hydroxymethylfurfural Electrooxidation

Stabilizing Ni³⁺ Species through High-Valence Molybdenum Introduction for 5-Hydroxymethylfurfural Electrooxidation

Electrochemical glucose-to-formic acid conversion coupled with alkaline hydrogen production over nanostructured CuCo₂O₄ catalysts

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Carbon layer confined Co–Ni bimetallic oxide heterojunctions for high-efficiency electrosynthesis of 2,5-furandicarboxylic acid

Abstract: Electrooxidation of 5-hydroxymethylfurfural (HMF) has been recognized as an efficient method for obtaining high value-added chemicals, so it is desirable to develop highly active and stable catalysts for electrocatalytic HMF...

Cited by 2 publications

References 43 publications

Stabilizing Ni3+ Species through High-Valence Molybdenum Introduction for 5-Hydroxymethylfurfural Electrooxidation

Stabilizing Ni3+ Species through High-Valence Molybdenum Introduction for 5-Hydroxymethylfurfural Electrooxidation

Electrochemical glucose-to-formic acid conversion coupled with alkaline hydrogen production over nanostructured CuCo2O4 catalysts

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Stabilizing Ni³⁺ Species through High-Valence Molybdenum Introduction for 5-Hydroxymethylfurfural Electrooxidation

Stabilizing Ni³⁺ Species through High-Valence Molybdenum Introduction for 5-Hydroxymethylfurfural Electrooxidation

Electrochemical glucose-to-formic acid conversion coupled with alkaline hydrogen production over nanostructured CuCo₂O₄ catalysts