2018
DOI: 10.1002/anie.201710509
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Catalysis of Carbon Dioxide Photoreduction on Nanosheets: Fundamentals and Challenges

Abstract: The transformation of CO into fuels and chemicals by photocatalysis is a promising strategy to provide a long-term solution to mitigating global warming and energy-supply problems. Achievements in photocatalysis during the last decade have sparked increased interest in using sunlight to reduce CO . Traditional semiconductors used in photocatalysis (e.g. TiO ) are not suitable for use in natural sunlight and their performance is not sufficient even under UV irradiation. Some two-dimensional (2D) materials have … Show more

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Cited by 415 publications
(285 citation statements)
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References 158 publications
(355 reference statements)
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“…[3,4] By using SCFs, the surfaces of graphene, rGO, or GO have been decorated with a variety of metal (such as Pt, [105,195] Ru, [105] Pd, [97,100,102,197] Ag, [84,198,216,217] Au, [100] Fe, [100] Ni, [100,105] PtRu, [199] PtFe, [107] and PtFeCo [200] ), metal oxide (such as ZnO, [99,101,218] Co 3 O 4 , [96] TiO 2 , [201,202,219] MoO 2 , [193] MnO 2 , [209] Al 2 O 3 , [215] and SnO 2 , [205] ), and metal sulfide (such as CdS [103] ) NPs with tunable sizes, loadings, and compositions. [3,4] By using SCFs, the surfaces of graphene, rGO, or GO have been decorated with a variety of metal (such as Pt, [105,195] Ru, [105] Pd, [97,100,102,197] Ag, [84,198,216,217] Au, …”
Section: Catalysismentioning
confidence: 99%
“…[3,4] By using SCFs, the surfaces of graphene, rGO, or GO have been decorated with a variety of metal (such as Pt, [105,195] Ru, [105] Pd, [97,100,102,197] Ag, [84,198,216,217] Au, [100] Fe, [100] Ni, [100,105] PtRu, [199] PtFe, [107] and PtFeCo [200] ), metal oxide (such as ZnO, [99,101,218] Co 3 O 4 , [96] TiO 2 , [201,202,219] MoO 2 , [193] MnO 2 , [209] Al 2 O 3 , [215] and SnO 2 , [205] ), and metal sulfide (such as CdS [103] ) NPs with tunable sizes, loadings, and compositions. [3,4] By using SCFs, the surfaces of graphene, rGO, or GO have been decorated with a variety of metal (such as Pt, [105,195] Ru, [105] Pd, [97,100,102,197] Ag, [84,198,216,217] Au, …”
Section: Catalysismentioning
confidence: 99%
“…The depletion of fossil fuel source with tremendous emissions of CO 2 , which is a main greenhouse gas, results in the increasing energy crisis and global warming issues, profoundly affecting human survival and development . Besides, water pollution, which is caused by organic contaminants, has become a great threat to human health .…”
Section: Introductionmentioning
confidence: 99%
“…The depletion of fossil fuel source with tremendous emis sions of CO 2 , which is a main greenhouse gas, results in the increasing energy crisis and global warming issues, pro foundly affecting human survival and development. [1] Besides, water pollution, which is caused by organic contaminants, has become a great threat to human health. [2] As a promising and powerful approach, photocatalysis, which occurs on the surface of semiconductors to convert simple molecules (i.e., H 2 O or CO 2 ) into solar fuels or degrade organic pollutants effectively, has attracted tremendous interests from scientists.…”
Section: Introductionmentioning
confidence: 99%
“…The true formation of products from CO 2 as carbon source can be evidenced by three general approaches: (1) by the stoichiometric detection of the byproduct oxygen; this is considered the best way, because it would also evidence that no sacrificial reagents are present and that the catalytic cycle is closed; (2) by 13 C‐labeling of CO 2 and a detection of 13 C‐labeled products, or (3) the verification of the absence of product formation in a blank experiment, in which under otherwise similar reaction conditions CO 2 has been replaced by an inert gas . It is acknowledged that the latter two possibilities do not at the same time evidence that the catalytic cycle is truly closed.…”
Section: Introductionmentioning
confidence: 99%