2010
DOI: 10.1007/s10562-010-0450-9
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Catalytic Oxidation of Chlorobenzene over MnO x /Al2O3-carbon Nanotubes Composites

Abstract: MnO x /Al 2 O 3 -carbon nanotubes (CNTs) composites prepared by hydrothermal method were characterized by XRD, SEM, TEM, TGA, BET, XPS and H 2 -TPR. Catalytic oxidation of chlorobenzene (CB) was conducted over the composites under gas hourly space velocity (GHSV) of 36000 h -1 and CB concentration of 2800 ppmv. For the catalyst with approximately 25 wt% CNTs and 10 at.% Mn, CB removal efficiencies reached up to 83.3 and 97.7% at 150 and 300°C, respectively. Moreover, no Cl species was detected over the used Mn… Show more

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Cited by 39 publications
(23 citation statements)
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“…A support with a high BET surface area can effectively generate more surface active sites and promote charge transfer, which is benecial for the catalytic performance. 21,46 Based on the XRD and N 2 adsorption results, it is most likely that the decreased catalytic efficiency of the decomposed sample can be attributed to the crushed special structure and the decreased surface area of the catalyst. From the comparative experimental results, the MOF was proven to be a potential supporting material for the impregnated Mn-Ce catalysts.…”
Section: Catalytic Performances Of the Decomposed Catalystsmentioning
confidence: 99%
“…A support with a high BET surface area can effectively generate more surface active sites and promote charge transfer, which is benecial for the catalytic performance. 21,46 Based on the XRD and N 2 adsorption results, it is most likely that the decreased catalytic efficiency of the decomposed sample can be attributed to the crushed special structure and the decreased surface area of the catalyst. From the comparative experimental results, the MOF was proven to be a potential supporting material for the impregnated Mn-Ce catalysts.…”
Section: Catalytic Performances Of the Decomposed Catalystsmentioning
confidence: 99%
“…In addition, CNTs are also good NO X adsorbents [21] and have a positive effect on the elimination of organic pollution [22,23]. This study reports the reduction of NO X with ammonia over the V 2 O 5 -MnO X /TiO 2 -CNTs plate-like catalyst in a fixed-bed flow-reactor.…”
Section: Introductionmentioning
confidence: 92%
“…Nitric oxide (NO) exhausted from waste incinerators, industrial boilers, engines, and automobiles can cause photochemical smog, acid rain, greenhouse effect and haze weather, which are harmful to the ecosystem and humanity [1][2][3][4][5] . Therefore, strict control of nitric oxide emission and removal processes was urgently needed.…”
Section: Introductionmentioning
confidence: 99%