2024
DOI: 10.1002/cssc.202401141
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Catalytic Pyrolysis of Polyethylene with Microporous and Mesoporous Materials: Assessing Performance and Mechanistic Understanding

Johan H. van de Minkelis,
Adrian H. Hergesell,
Jan C. van der Waal
et al.

Abstract: Testing the catalytic performance for the catalytic pyrolysis of plastic waste is hampered by mass transfer limitations induced by a size mismatch between the catalyst′s pores and the bulky polymer molecules. To investigate this aspect, the catalytic behaviour of a series of microporous and mesoporous materials was assessed in the catalytic pyrolysis of polyethylene (PE). More specifically, a mesoporous material, namely sulfated zirconia (Zr(SO4)2) on SBA‐15, was synthesized to increase the pore accessibility,… Show more

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