Catalytic stereoselective synthesis of cyclopentanones from donor–acceptor cyclopropanes and <i>in situ</i>-generated ketenes

Mitra, Shubhanjan; Connolly, Sophie M.; Ayidi, Saud; Mondal, Mukulesh; Panda, Manashi; Kelly, Brian G.; Kerrigan, Nessan J.

doi:10.1039/d4ob01313a

Org. Biomol. Chem.

2024

DOI: 10.1039/d4ob01313a

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Catalytic stereoselective synthesis of cyclopentanones from donor–acceptor cyclopropanes and in situ-generated ketenes

Shubhanjan Mitra,

Sophie M. Connolly,

Saud Ayidi

et al.

Abstract: A dual InBr3-EtAlCl2 Lewis acidic system was found to be optimal for promoting the diastereoselective (3 + 2)-cycloaddition of donor-acceptor cyclopropanes with in situ-generated ketenes to form cyclopentanones. The desired...

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Catalytic stereoselective synthesis of cyclopentanones from donor–acceptor cyclopropanes and in situ-generated ketenes

Abstract: A dual InBr3-EtAlCl2 Lewis acidic system was found to be optimal for promoting the diastereoselective (3 + 2)-cycloaddition of donor-acceptor cyclopropanes with in situ-generated ketenes to form cyclopentanones. The desired...

Cited by 0 publications

References 52 publications

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