“…Experimental investigations addressing location, compositions, structure and geometrical features of segregates in sample ingots were accompanied by theoretical considerations (e.g., CALPHAD approaches realized using the Thermo-Calc software package), finally leading to a model of freckle segregation formation which integrates, among others, geometric, thermodynamic, fluid dynamic and compositional aspects as well as composition-dependent viscosity levels. As a result, a threshold for freckle formation was suggested in terms of a relative Rayleigh number limit for the material in question [379].…”