The 1.315 µm [I(2P1/2) → I(2P3/2)] transition of atomic iodine in the chemical oxygen–iodine laser (COIL) is pumped by sequential reactions of I2 and I with O2(1Δ). In electrically pumped systems (eCOILs), electron impact excitation of O2 produces the O2(1Δ) and also produces O atoms through dissociative excitation. The O atoms, through reactions with I2, I(2P1/2) and I(2P3/2), lead to dissociation of I2, quenching of the upper laser level and removal of the lower laser level. While dissociating I2 is potentially beneficial, quenching of the upper laser level is detrimental and so management of the O atom density is necessary to maximize laser gain. In this regard, NO and NO2 additives have been used to manage the O atom density by cyclically reacting with O and I. In this paper, results from a computational investigation of eCOIL systems using plug flow and two-dimensional models are discussed where NO and NO2 additives are used. The system is a flowing plasma sustained in He/O2/NO mixtures with downstream injection of NO2 followed by injection of I2. We found that addition of NO and NO2 is effective in managing the density of O atoms and maximizing gain by minimizing quenching of the upper laser level. We found that by optimizing the additives, laser gain can be maximized even though O2(1Δ) densities may be lower due to the management of quenching and dissociation reactions.