2013
DOI: 10.1063/1.4802915
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Characterization of submicron-sized CO2 clusters formed with a supersonic expansion of a mixed-gas using a three-staged nozzle

Abstract: The size of CO2 clusters, produced in a supersonic expansion of a mixed-gas of CO2/He or CO2/H2 through a three-staged conical nozzle designed based on the Boldarev's model, has been evaluated by measuring the angular distribution of light scattered from the clusters. The data are analyzed utilizing the Mie scattering theory, and the sizes of CO2 clusters are estimated as 0.22 μm and 0.25 μm for the cases of CO2/He and CO2/H2 gas mixtures, respectively. The results confirm that the Boldarev's model is reliable… Show more

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Cited by 26 publications
(19 citation statements)
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“…The capability of this model for the gas density has been demonstrated. 19,21,23 In this work, the gas jets of eighteen conical nozzles with the same throat diameter d of 0.5 mm under five gas backing pressures were simulated for the on-axis atom number density. As examples, the results about density at the gas backing pressure of 50 bars are shown in Fig.…”
Section: Resultsmentioning
confidence: 99%
See 1 more Smart Citation
“…The capability of this model for the gas density has been demonstrated. 19,21,23 In this work, the gas jets of eighteen conical nozzles with the same throat diameter d of 0.5 mm under five gas backing pressures were simulated for the on-axis atom number density. As examples, the results about density at the gas backing pressure of 50 bars are shown in Fig.…”
Section: Resultsmentioning
confidence: 99%
“…Thus one a Author to whom correspondence should be addressed: kimd@postech.ac.kr 2158-3226/2015/5(10)/107220/7 5, 107220-1 © Author(s) 2015 expects the cluster size deviation when the scaling law is used to estimate the cluster size under a high gas backing pressure. Up to now, there have existed many papers about the investigation of the gas jet and its cluster size, [9][10][11][12][13][14][15][16][17][18][19] and there have been papers reporting the cluster size deviation from the size expected by the scaling laws 20,21 and some works concerned about the understanding of the deviation. 22 In Ref.…”
Section: Introductionmentioning
confidence: 99%
“…17 Other researchers measured the value of g using Mie scattering from very large clusters (several hundreds of nanometers diameter). 18,19 However, this Mie scattering technique would not be applicable for the much smaller clusters in our work (up to few tens of nanometers diameter).…”
Section: Introductionmentioning
confidence: 90%
“…The capability of this model for the spatial distribution of gas density has been demonstrated. 16,18,19 The 2D hydrodynamic model reproduces the spatial structure of the gas jet, including the rarefaction waves at the edges of the jet, and it is possible to evaluate the diameter on the base of the simulated results by introducing a threshold density value. Similarly to the definition of gas diameter in Ref.…”
Section: Aip Advances 6 115015 (2016)mentioning
confidence: 99%
“…3,4 The production of a gas jet and its characterization have attracted interests and been extensively studied. [5][6][7][8][9][10][11][12][13][14][15][16][17][18][19] Usually, a supersonic clustered gas jet can be produced by the adiabatic expansion of gas under a high backing pressure through a conical nozzle into vacuum. The dimension of a gas jet is an important parameter for the determination of interaction length.…”
Section: Introductionmentioning
confidence: 99%