“…However, the variation of these ratios with volcanic activity differs among volcanoes: increases (e.g., Hirabayashi et al, 1982;Aiuppa et al, 2004) and decreases (e.g., Noguchi and Kamiya, 1963;Taran et al, 2002;Duffel et al, 2003) of these ratios are reported to be associated with increasing volcanic activity. In the case of Aso volcano, high HCl/SO 2 ratios were observed soon after intense eruptive activities, and subsequently decreased after the activities ceased (Iwasaki et al, 1962;Ossaka et al, 1978Ossaka et al, , 1984. Although these observations described sporadically the relation between the HCl/SO 2 ratio and volcanic activity, continuous and longer observation is needed to further understand this relation.…”