We study the low-temperature properties of a classical Heisenberg model with site-random interlayer couplings on the cubic lattice. This model is introduced as a simplified effective model of Sr(Fe 1−x Mn x )O 2 , which was recently synthesized. In this material, when x = 0.3, (πππ) and (ππ0) mixed ordering is observed by neutron diffraction measurements. Using Monte Carlo simulations, we find an exotic bulk spin structure that explains the experimentally obtained results. We name this spin structure the "random fan-out state." The mean-field calculations provide an intuitive understanding of this phase being induced by the site-random interlayer couplings. Since Rietveld analysis assuming the random fan-out state agrees well with the neutron diffraction pattern of Sr(Fe 0.7 Mn 0.3 )O 2 , we conclude that the random fan-out state is reasonable for the spin-ordering pattern of Sr(Fe 0.7 Mn 0.3 )O 2 at the low-temperature phase. PACS number(s): 75.50. Lk, 75.40.Mg, 28.20.Cz Sr(Fe 0.7 Mn 0.3 )O 2 using the spin configuration obtained from Monte Carlo simulations at low temperature.
A. Robustness of random fan-out stateIn this section, we discuss the relationship between decision rules of interactions and the spin-ordering pattern. In general, the spatial average of interlayer random interactions J and its fluctuation J corresponding to the random fields depend on the signs and absolute values of interactions:where J AA , J AB , and J BB denote the interactions between A-A, A-B, and B-B along the interlayer direction, respectively. Then, the spatial average of effective interaction between the NNLs, J nnl , is given by(36) Here, we assume that J AA is always AF and the absolute values of interactions are the same or zero. Then, the four rules in Table III are all possible decision rules of interactions where FM and AF interactions exist and J nnl < 0 regardless of x. Note that rule 1 is adopted in the previous sections. Under these rules and using Monte Carlo simulations and meanfield calculations, we find the appearance of the mixed phase, where the spin-ordering pattern is the random fan-out state. Furthermore, we also find that (πππ) and (ππ0) magnetic peaks develop at the same temperature and the angle between 214408-8 RANDOM FAN-OUT STATE INDUCED BY SITE-RANDOM . . .