Compared with the domain wall motion in a ferromagnetic nanowire, the chiral soliton motion could reach a much larger velocity at a much smaller current density. [9,11] The metallic chiral magnets that can host CSL are very rare. As far as we know, the formation of CSL in metallic chiral magnets has been only observed in Cr 1/3 NbS 2 and YbNi 3 Al 9 . [2,3,12,13] As the stability of chiral magnetic solitons is determined by the Dzyaloshinskii-Moriya (DM) interaction and the velocity of soliton motion is controlled by the non-adiabatic torque, searching for new chiral magnets associate with strong DM interaction and large non-adiabatic torque is of great importance in the emerging field of solitonics. [2,3,8,9] Among the various candidates, the magnetic ion (M = Cr, Mn, Fe, Co, and Ni) intercalated M 1/3 TaS 2 stands out because the parent compound TaS 2 has large spin-orbit coupling (SOC) and hosts a rich collection of exotic states including the Mott state, charge density wave, and quantum spin liquid. [14][15][16] As the magnetic ions insert into TaS 2 , the ordering of magnetic ions in M 1/3 TaS 2 results in a (1/3, 1/3, 0) superstructure with a chiral space group of P6 3 22. [17] The strong SOC and the chiral lattice structure of M 1/3 TaS 2 could induce strong DM interaction and large non-adiabatic torque, since the strength of DM interaction and non-adiabatic torque both are proportional to the SOC constant. [18,19] In the family of M 1/3 TaS 2 , only Fe 1/3 TaS 2 has been confirmed as a chiral magnet. [17,20] Nevertheless, the extremely large orbital magnetic moment of Fe 2+ ions yields the gigantic easy-axis magnetocrystalline anisotropy and brings on the Ising-type ferromagnetic structure in Fe 1/3 TaS 2 . [17,21] The crystal growth and characterization of several other M 1/3 TaS 2 have been studied as early as the 1980s, yet whether the crystals possess chiral lattice structure and chiral magnetism are in question. [22][23][24] For example, the Cr 1/3 TaS 2 has been reported to exhibit a trivial ferromagnetic (FM) transition near 115 K without any hints of chiral features. [22][23][24][25] In this work, we report the magneto-transport properties and magnetic phase diagrams of Cr 1/3 TaS 2 single crystals. In contrast with the reported trivial FM transition, our Cr 1/3 TaS 2 single crystals exhibit a chiral helimagnetic (CHM) transition near 140 K. The conducting electrons interact with the CHM and CSL orders, giving rise to the nontrivial magnetoresistance (MR) in Cr 1/3 TaS 2 . The normalized magnetic moment and Cr 1/3 TaS 2 -a candidate of chiral magnet-has been reported as a trivial ferromagnetic material. In contrast, the Cr 1/3 TaS 2 single crystals exhibit a chiral helimagnetic (CHM) transition near 140 K. The magnetic moment versus magnetic field curves reveal a CHM-chiral soliton lattice (CSL)-forced ferromagnetic (FFM) transition in the magnetic ordered state. The conducting electrons interact with the CHM and CSL orders, giving rise to the nontrivial magnetoresistance (MR) in the Cr 1/3 TaS 2 ...