CO<sub>2</sub> conversion to CO <i>via</i> plasma and electrolysis: a techno-economic and energy cost analysis

Osorio-Tejada, Jose; Escriba-Gelonch, Marc; Vertongen, Rani; Bogaerts, Annemie; Hessel, Volker

doi:10.1039/d4ee00164h

Energy Environ. Sci.

2024

DOI: 10.1039/d4ee00164h

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CO₂ conversion to CO via plasma and electrolysis: a techno-economic and energy cost analysis

Jose Osorio-Tejada,

Marc Escriba-Gelonch,

Rani Vertongen

et al.

Abstract: Electrification and carbon capture technologies are essential for achieving net-zero emissions in the chemical sector. A crucial strategy involves converting captured CO2 into CO, a valuable chemical feedstock. This study...

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2024

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Cited by 3 publications

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Sustainability assessment of plasma-based and electrolytic CO2 conversion to CO

Escribà-Gelonch,

Osorio-Tejada,

Vertongen

et al. 2024

Journal of Cleaner Production

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Sustainability assessment of plasma-based and electrolytic CO2 conversion to CO

Escribà-Gelonch,

Osorio-Tejada,

Vertongen

et al. 2024

Journal of Cleaner Production

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Enhancing CO2 conversion in a temperature-controlled DBD plasma reactor with HKUST-1 catalyst: Water removal and CuO/Cu2O-derived approach

Hatami,

Khani,

Shokri

2024

Results in Engineering

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Salophen-Type Schiff Bases Functionalized with Pyridinium Halide Units as Metal-Free Catalysts for Synthesis of Cyclic Carbonates from Carbon Dioxide and Terminal Epoxides

Kawka,

Bester,

Bukowska

et al. 2024

Catalysts

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Objectives: Salophen-type Schiff bases functionalized with 4-(dimethylamino)pyridinium halide units are shown to be effective single-component catalysts for the synthesis of cyclic carbonates from terminal epoxides and carbon dioxide. Methods: Using one of such trifunctional organocatalysts, epichlorohydrin could be selectively converted to the target cyclic carbonate under 2 bar of CO2 at 120 °C. Results: Over 80% conversion of E3 was then observed when organocatalyst S3 was used in the amount of 0.5 mol% (TON = 156) and even the use of 0.05 mol% S3 guaranteed almost 50% conversion of E3 to C3 (TON = 893). Conclusions: The presence of tertiary amine units in the molecules of these homogeneous organocatalysts proved to be crucial for the catalytic activity of developed organocatalysts. However, their catalytic activity was also supported by the presence of acidic phenolic units and halide ions as Lewis bases. Some closely related compounds were found to be clearly less active or inactive catalytically under the applied reaction conditions.

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CO₂ conversion to CO via plasma and electrolysis: a techno-economic and energy cost analysis

Abstract: Electrification and carbon capture technologies are essential for achieving net-zero emissions in the chemical sector. A crucial strategy involves converting captured CO2 into CO, a valuable chemical feedstock. This study...

Cited by 3 publications

References 121 publications

Sustainability assessment of plasma-based and electrolytic CO2 conversion to CO

Sustainability assessment of plasma-based and electrolytic CO2 conversion to CO

Enhancing CO2 conversion in a temperature-controlled DBD plasma reactor with HKUST-1 catalyst: Water removal and CuO/Cu2O-derived approach

Salophen-Type Schiff Bases Functionalized with Pyridinium Halide Units as Metal-Free Catalysts for Synthesis of Cyclic Carbonates from Carbon Dioxide and Terminal Epoxides

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Resources

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CO2 conversion to CO via plasma and electrolysis: a techno-economic and energy cost analysis

Abstract: Electrification and carbon capture technologies are essential for achieving net-zero emissions in the chemical sector. A crucial strategy involves converting captured CO2 into CO, a valuable chemical feedstock. This study...

Cited by 3 publications

References 121 publications

Sustainability assessment of plasma-based and electrolytic CO2 conversion to CO

Sustainability assessment of plasma-based and electrolytic CO2 conversion to CO

Enhancing CO2 conversion in a temperature-controlled DBD plasma reactor with HKUST-1 catalyst: Water removal and CuO/Cu2O-derived approach

Salophen-Type Schiff Bases Functionalized with Pyridinium Halide Units as Metal-Free Catalysts for Synthesis of Cyclic Carbonates from Carbon Dioxide and Terminal Epoxides

Contact Info

Product

Resources

About

CO₂ conversion to CO via plasma and electrolysis: a techno-economic and energy cost analysis