Abstract. This study analyzed the aerosol optical properties
derived by SKYRAD.pack versions 5.0 and 4.2 (referred to as V5.0 and V4.2)
using the radiometer measurements over Qionghai and Yucheng in China, two
new sites of the sky radiometer network (SKYNET). As V5.0 uses an a priori
size distribution function (SDF) of a bimodal log-normal function, the
volume size distribution retrieved by V5.0 presented bimodal patterns with a
0.1–0.2 µm fine particle mode and a 3.0–6.0 µm coarse particle
mode both over Qionghai and Yucheng. The differences in the volume size
distributions between the two versions were very large for the coarse mode
with a radius of over 5 µm. The single scattering albedos (SSAs)
by V5.0 correlated with SSAs by V4.2 with R=0.88, 0.87, 0.90, 0.88, and
0.92 at wavelengths of 400, 500, 670, 870, and 1020 nm over Qionghai,
respectively. The correlation coefficients were around 0.95, 0.95, 0.96,
0.94, and 0.91 at the five channels in Yucheng. An error of ±5 %
for the solid view angle (SVA) introduced about ±2 % differences in
retrieved SSA values both by V4.2 and V5.0. An error of ±50 % for
ground surface albedo (Ag) caused about 1 % averaged differences in
retrieved SSA values by the two versions. With the atmospheric pressure
(PRS) increased by 1 %, 2 %, 3 %, and 4 %, the averaged changes in
SSAs did not exceed 0.8 % both by V4.2 and V5.0. The SSA differences at
500 nm between the two versions decreased, while aerosol optical depths (AODs) increased over both
sites. The seasonal variability of the aerosol properties over Qionghai and
Yucheng was investigated based on SKYRAD.pack V5.0. The seasonal averaged
AOD over Qionghai had higher values in spring, winter, and autumn and lower
values in summer. The AOD averages were commonly higher in summer and spring
than in winter and autumn in Yucheng. The lowest seasonal averaged SSAs were
both observed in winter at the two sites. The fraction of the fine aerosol
particles was much smaller in summer than in other seasons over Qionghai;
the volume fraction of the coarse-mode particle in Yucheng had much larger
values compared to the fine-mode particle in all seasons. The validation
results provide valuable references for continued improvement of the
retrieval algorithms of SKYNET and other aerosol observational networks.