Numerous empirical studies have demonstrated that street trees not only reduce dust pollution and absorb particulate matter (PM) but also improve microclimates, providing both ecological functions and aesthetic value. However, recent research has revealed that street tree canopy cover can impede the dispersion of atmospheric PM within street canyons, leading to the accumulation of street pollutants. Although many studies have investigated the impact of street trees on air pollutant dispersion within street canyons, the extent of their influence remains unclear and uncertain. Pollutant accumulation corresponds to the specific characteristics of individual street canyons, coupled with meteorological factors and pollution source strength. Notably, the characteristics of street tree canopy cover also exert a significant influence. There is still a quantitative research gap on street tree cover impacts with respect to pollution and dust reduction control measures within street spaces. To improve urban traffic environments, policymakers have mainly focused on scientifically based street vegetation deployment initiatives in building ecological garden cities and improving the living environment. To address uncertainties regarding the influence of street trees on the dispersion of atmospheric PM in urban streets, this study reviews dispersion mechanisms and key atmospheric PM factors in urban streets, summarizes the research approaches used to conceptualize atmospheric PM dispersion in urban street canyons, and examines urban plant efficiency in reducing atmospheric PM. Furthermore, we also address current challenges and future directions in this field to provide a more comprehensive understanding of atmospheric PM dispersion in urban streets and the role that street trees play in mitigating air pollution.