GaN-based LEDs were fabricated on patterned-sapphire substrates with various pyramidal-pattern coverage percentages (31-81%). Three distinguish stages are observed in the behavior of the light out-put power against coverage percentage. By etching-pit density measurement, dislocation density is found to be independent with coverage percentage. The light extraction efficiency (LEE) should be the main mechanism for the enhancement in the light out-put power. LEE would be enhanced, when the pattern coverage is less than 39% or over 67%. The light extraction efficiency remains similar, when the pattern coverage in between 39% ∼ 67%.The sapphire substrate patterning technique has been widely used to improve the external quantum efficiency (EQE) of GaN-based LEDs. 1-10 The improvement obtained using the patterned-sapphire substrate (PSS) technique includes the enhancements of both the internal quantum efficiency (IQE) and light extraction efficiency (LEE). The LEE is enhanced because of the patterns on the PSS act to destroy the TIR (Total Internal Reflection) effect at the GaN/sapphire interface. 1, 3, 4 Several published literatures have pointed out that the light extraction efficiency could be increased by using periodic or non-periodic micron-sized patterning on sapphire substrate. 11-16 On the other hand, the patterns on the PSS can reduce the threading dislocations in the GaN epitaxial layers owing to the possible lateral growth of the GaN epi-layer. 2,5,6,8,17 Some recent studies indicated that the use of nano-scale patterned sapphire substrate leads to increase in IQE, which is resulted from the significant reduction in the threading dislocation density (two-orders of magnitude reduction) and reduction in the fraction of the screw dislocation density. 18-21 Besides, some researchers also indicate that IQE can be improved by QW designing (for examples, non-polar QW and large overlap QW). [22][23][24][25][26][27][28][29] Generally, it seems that the greater the pattern coverage created on the PSS, the higher the LEE would be. 30 However, there so far been no any experimental study or systematically investigation of the effect of the pattern coverage of the PSS on the and LEE. Another key issue that is not yet well understood is how does the pattern coverage (or c-plane coverage) influence the IQE of a GaN-based LED on the PSS. In this study, a mask-free wet-etching process is used to produce a so-called naturally patterned-sapphire substrate (n-pss). 31 By varying the etching time and temperature, different amount of pyramidal pattern coverage can be created on the n-pss wafers. The effect of the pyramidal pattern coverage on the IQE and LEE of the GaN epi-layers can be studied.The mask-free wet-etching process used to produce the pyramidal n-pss wafers is described in detail below. Before the wet-etching process, a PECVD (Plasma Enhanced Chemical Vapor Deposition) SiO 2 layer was deposited on the back-side of the c-plane sapphire wafers to prevent the back-side of sapphire wafers from being etched. The flat back-...