where the amount generated in each color is dependent on the phase mismatch value of the process and the length of the nonlinear interaction between the waves [4]. By definition, SPDC is a nonlinear process in which the frequencies of the photon pairs are lower than that of the pump wave. For this reason, conventional generation of photon pairs in the visible optical regime typically requires ultraviolet pump frequencies. The use of ultraviolet light in such schemes is very challenging because of the large phase mismatch between the waves, resulting in very poor conversion efficiency. Furthermore, several highly efficient nonlinear crystals-LiNbO 3 and KTiOPO 4 -are opaque in the ultraviolet range and therefore cannot be used.One way to overcome such difficulties is to perform SPDC followed by an upconversion process that allows for frequency conversion of light from near-infrared to visible. In addition, nonlinear frequency conversion of photon pairs provides a wavelength flexibility that is important for many applications, including the realization of practical quantum communication networks [5]. Yet, as the generation of SPDC spectra typically spans a large bandwidth, the conventional approach of optical upconversion in a nonlinear device fails due to the narrowband nature of the frequencyconversion process in a perfect phase-matched interaction [1, 6]. Thus, for broadband photon pair generation, the total nonlinear efficiency of such sequential processes is commonly quite poor. However, it is possible to tradeoff efficiency for high phase-matching bandwidth by using carefully designed QPM crystals. But owing to the high dispersion of most quasi-phase-matched crystals, which increases significantly in the visible regime, the required width of the QPM pattern for phase-matching compensation is very small and is currently beyond the limits of most fabrication methods.Abstract We experimentally demonstrate a method for creating broad bandwidth photon pairs in the visible spectral region, centered at a frequency that is higher than that of the initial pump source. Spontaneous down conversion of a narrowband 1053 nm pulsed Nd:YLF laser is followed by highly efficient upconversion in adiabatic nonlinear frequency-conversion process. Photon pairs are generated from 693 to 708 nm, and the complete conversion process occurs within a single monolithic 5-cm-long stoichiometric lithium tantalate nonlinear crystal. We have characterized the dependence of this structure with respect to pump intensity and crystal temperature.Spontaneous parametric down conversion (SPDC) plays a key role in nonlinear and quantum optics as it enables amplification of broadband, tunable light in optical parametric oscillators and the reliable generation of entangled photon pairs [1,2]. SPDC originates from the stimulation of random vacuum fluctuations, induced by a strong pump in a optical parametric generation (OPG) process [3]. In this process, the pump photon at ω p spontaneously splits into two photons, the signal at ω 1 and the idler at ω ...