The African upper mantle is diverse, featuring several cratonic roots, active and magmatic continental rifting, abundant intra‐plate volcanism, and several oceanic hotspots offshore. Relatively small‐scale mantle convection processes, some possibly related to lithospheric thickness variations, have been proposed to account for patterns of volcanism and topography. A key constraint on such features and processes can be found via seismic anisotropy, but limited coverage of seismograph stations across the continent has resulted in sparse observations. Quasi‐Love waves, produced by scattering of Love to Rayleigh energy at lateral gradients in upper mantle seismic anisotropy, can provide information about seismic anisotropy well away from seismograph stations. We catalog 525 observations of Quasi‐Love waves across the region and back‐project to scattering points, revealing locations of lateral gradients in upper mantle seismic anisotropy. Quasi‐Love wave scattering occurs at craton edges, likely due to the contrast between lithospheric and asthenospheric anisotropy, and close to ancient orogenic belts, indicating changes in fossilized lithospheric anisotropy from past collisional events. Scattering surrounding the proposed Al‐Kufrah cratonic remnant in north‐east Africa supports its existence as cratonic lithosphere. Scattering also occurs below thin lithosphere, suggesting deviations in asthenospheric flow patterns (such as localized upwellings), notably beneath the East African Rift, oceanic hotspot tracks, and the Cameroon Volcanic Line. Quasi‐Love scattering is abundant in the Indian Ocean and beneath Madagascar, consistent with small‐scale dynamic processes in the asthenosphere that likely relate to the complex rifting history of this ocean basin and the dispersed micro‐continents within.