“…These combined technological improvements have allowed the SELENE Spectral Profiler and Multiband Imager (MI) and the Chandrayaan‐1 Moon Mineralogy Mapper (M 3 ) to unambiguously identify Fe‐bearing crystalline plagioclase across the lunar surface based on its unique 1.25 µm absorption band [ Burns , , ; Adams and McCord , ; Adams and Goullaud , ]. Pure crystalline plagioclase has now been identified in widespread locations across the lunar surface: around impact basins, in massifs in the Inner Rook Mountains of Orientale, and in the central peaks, walls, floor, and ejecta of craters [ Matsunaga et al , ; Ohtake et al , ; Pieters et al , ; Dhingra et al , ; Donaldson Hanna et al , ; Yamamoto et al , ; Cheek et al , ]. While previous NIR laboratory studies have suggested that the band depth and center position of the 1.25 µm feature may vary with Fe and An contents [ Bell and Mao , ; Adams and Goullaud , ; Cheek et al , , ], the relationship between NIR spectral properties of plagioclase and its composition (An#) has yet to be quantified.…”