Carbon foams (CFms) are of crucial importance in electrical and mechanical devices due to their high thermal conductivity used for eliminating high heat flow and maintaining low temperatures [1]. The most common CFms are types of aluminum alloys, copper and diamond. However, the mechanical properties of metal-based heat sink materials are difficult to control at temperatures over 550°C [2,3]. Thus, CFms are actively investigated as heat sink materials because of their good properties, such as high thermal stability, high thermal/electrical conductivity, low density, high porosity and high specific surface area [4,5]. CFms are suitable materials for applications in phase-change materials, such as in latent heat thermal energy storage and lithium-ion batteries [6][7][8][9].CFms are prepared from thermoplastic graphitizable precursors, such as petroleum-derived, coal-derived and mesophase pitch (MP). In particular, MP has been widely used as an appropriate precursor for high-performance carbon materials due to its attractive properties, i.e., high coke yield, low softening point, and high fluidity [10]. Previous processes used a blowing technique, or pressure release, to produce foam from MP. These manufacturing techniques have many disadvantages: the volume fraction of generated cells cannot be precisely controlled, and controlling the shape and distribution of cells is difficult, if not impossible [11]. To better control and tailor the structure of such foams, polymer template methods are actively being researched. Hydrogel template methods are suitable for preparing high-strength CFms due to their large quantities of carbon precursors and the pressure generated through hydrogel shrinkage via heat treatment [10,12]. However, their mechanical strengths are low because of their high porosities.One method for improving the mechanical strength of CFms is adding fillers with a high mechanical strength. Several additives have been used as fillers, including carbon nanofibers, short carbon fibers, graphite and graphene nanosheets [13][14][15][16][17][18][19][20][21][22]. In particular, graphite has beneficial properties that include high lubricating ability, heat resistance, corrosion resistance and thermal/electrical conductivity. It has been widely applied in various fields as a highly functional component with efficient properties. Additionally, the theoretical thermal conductivity of graphite is high, with values ranging from 3000 to 5000 W/mK, and its mechanical strength is 1100 GPa [23,24]. The thermal/mechanical properties of CFms could be improved by the addition of carbon nanofillers with good thermal/mechanical properties through the formation of network structures comprising CFms and carbon nanofillers. Furthermore, carbon nanofillers can be carbon-coated (C-coated) to improve the interfacial bonding with metal. For example, Katzman [25] showed that carbon fibers could be C-coated using amorphous pitch to improve the interfacial bonding with metal oxide and prepare a carbon-fiber-reinforced metal-matrix compo...