We present ideas aimed at bringing revolutionary changes on architectures and buildings of tomorrow by radically advancing the technology for the building material concrete and hence building components. We propose that by using nanotechnology we could embed computation and sensing directly into the material used for construction. Intelligent concrete blocks and panels advanced with stimuli-responsive smart paints are the core of the proposed architecture. In particular, the photo-responsive paint would sense the buildings internal and external environment while the nano-materialconcrete composite material would be capable of sensing the building environment and implement massive-parallel information processing resulting in distributed decision making. A calibration of the proposed materials with in-materio suitable computational methods and corresponding building in-formation modelling, computer-aided design and digital manufacturing tools could be achieved via models and prototypes of information processing at nano-level. The emergent technology sees a building as high-level massiveparallel computer -assembled of computing concrete blocks. Based on the generic principles of neuromorphic computation and reservoir computing we envisage a single building or an urban quarter to turn into a large-scale sensing substrate. It could behave as a universal computer, collecting and processing environmental information in situ enabling appropriate data fusion. The broad range of spatio-temporal effects include infrastructural and human mobility, energy, bio-diversity, digital activity, urban management, art and socializing, robustness with regard to damage and noise or real-time monitoring of environmental changes. The proposed intelligent architectures will increase sustainability and viability in digitised urban environments by decreasing information transfer bandwidth by e.g, utilising 5G networks. The emergence of socio-cultural effect will create a cybernetic relationship with our dwellings and cities.