CoNi Nanoparticles Supported on Hierarchical SAPO-34 Zeolite as a Catalyst for the Hydrolytic Dehydrogenation of Ammonia Borane

Cong, Wenwen; Zhang, Hongxia; Bing, Liancheng; Wang, Fang; Han, Dezhi; Wang, Guangjian

doi:10.1021/acsanm.3c04198

ACS Appl. Nano Mater.

2023

DOI: 10.1021/acsanm.3c04198

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CoNi Nanoparticles Supported on Hierarchical SAPO-34 Zeolite as a Catalyst for the Hydrolytic Dehydrogenation of Ammonia Borane

Wenwen Cong,

Hongxia Zhang,

Liancheng Bing

et al.

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Cited by 4 publications

References 49 publications

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In situ construction of Co–Mo2C on N-doped carbon for efficient hydrogen evolution from ammonia borane hydrolysis

Wu,

Liu,

Liu

et al. 2025

International Journal of Hydrogen Energy

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In situ construction of Co–Mo2C on N-doped carbon for efficient hydrogen evolution from ammonia borane hydrolysis

Wu,

Liu,

Liu

et al. 2025

International Journal of Hydrogen Energy

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Alkaline titanium carbide (MXene) engineering ultrafine non-noble nanocatalysts toward remarkably boosting hydrogen evolution from ammonia borane hydrolysis

Qin,

Tang,

et al. 2025

Journal of Alloys and Compounds

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Fabrication of Nano Pt–Co–Cu Sites in the Heterostructured Catalysts for Hydrogen Generation

Li,

Liu,

Zhang

et al. 2024

ACS Appl. Nano Mater.

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Ammonia borane hydrolysis for hydrogen production is considered as one of the most promising methods in the energy field. Rational design of both efficient and cost-effective catalysts for hydrogen generation is desirable but is still a challenge. Herein, we constructed interfacial Pt−Co−Cu sites in nanocatalysts for boosting hydrogen generation from ammonia borane hydrolysis. The ultrafine Pt nanoparticles were well dispersed on the CoCu-NC support, which was prepared by using the Cu-modified ZIF-67. The synergistic effects of multiple sites are responsible for the activation of H 2 O and NH 3 BH 3 molecules, which improved the catalytic activity in ammonia borane hydrolysis reaction. The effects of Pt and Cu loadings on the catalytic activity were investigated, and the dynamics data of the dehydrogenation reaction were also measured. The turnover frequency (TOF) value of the optimized catalyst is as high as 1636.28 min −1 at 298 K with addition of 0.44 M NaOH, and the prepared catalysts also presented the excellent recycling performance. This work provided a prospect to design heterostructured nanocatalysts for efficiently improving the hydrogen generation rate.

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CoNi Nanoparticles Supported on Hierarchical SAPO-34 Zeolite as a Catalyst for the Hydrolytic Dehydrogenation of Ammonia Borane

Cited by 4 publications

References 49 publications

In situ construction of Co–Mo2C on N-doped carbon for efficient hydrogen evolution from ammonia borane hydrolysis

In situ construction of Co–Mo2C on N-doped carbon for efficient hydrogen evolution from ammonia borane hydrolysis

Alkaline titanium carbide (MXene) engineering ultrafine non-noble nanocatalysts toward remarkably boosting hydrogen evolution from ammonia borane hydrolysis

Fabrication of Nano Pt–Co–Cu Sites in the Heterostructured Catalysts for Hydrogen Generation

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