As a very serious problem for control systems, actuator saturation often leads to an unstable system. The maneuvering flight of quadrotors may lead to actuator saturation, which commonly affects the flight quality, including trajectory-tracking accuracy. Quadrotors usually adopt double-closed-loop control, of which the outer loop is the position control used to calculate the desired attitude angle and the inner loop is the attitude control used to generate control actions for the vehicle. To address actuator saturation during the maneuvering flight of quadrotors, an attitude controller based on the conditioned super-twisting algorithm (CSTA) was designed. The sign functions in CSTA were replaced by a hyperbolic tangent function, which suppresses the chattering of CSTA. In order to improve the rapidity of the improved controller, the tanh-CSTA (TCSTA), a gain adjustment factor was utilized. The rapidity and smoothness of the controller can be satisfied by adjusting the gain factor. Additionally, a sliding surface was designed according to the characteristics of the quadrotor control structure, so that the TCSTA controller can be applied to the second-order system. The performances of the designed improved controller were simulated using MATLAB, and the results showed that the designed controller is more robust than the PID controller. Moreover, compared with the CSTA controller, the chattering of the designed controller was obviously suppressed without reducing the control accuracy.