2024
DOI: 10.1002/batt.202400558
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Constructing a Spider‐Web Polymer Blocking Layer on Separator for the High‐Loading Li‐S Battery

Qian Zhang,
Jiajun Wan,
Qingping Gao
et al.

Abstract: The cycling performance of high‐loading Li−S batteries is still puzzled by the serious shuttle effect of polysulfides. Modifying the commercial separator with polysulfide anchoring materials has been demonstrated as an economical and effective approach to block the polysulfide shuttle. Herein, a cobweb‐like polymer polysulfide‐blocking layer has been constructed via crosslinking between lithium polysilicate (LP) inorganic oligomer and tannic acid (TA) dendritic polymer. Owing to the strongly polar Si−O and Si=… Show more

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