2024
DOI: 10.1002/agt2.669
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Constructing benzothiadiazole‐based donor‒acceptor covalent organic frameworks for efficient photocatalytic H2 evolution

Yanchang Huang,
Bin Gao,
Qihang Huang
et al.

Abstract: Donor‒acceptor covalent organic frameworks (D‒A COFs) have been regarded as promising materials for photocatalytic water splitting because of their tunable band gaps. However, their efficiency is hindered by fast charge recombination and low photostability. Herein, we proposed a donor structural engineering strategy for improving the photocatalytic activity of D‒A COFs to tackle these problems. Two benzothiadiazole‐based D‒A COFs (DHU‐COF‐BB and DHU‐COF‐BP) with distinct donors were prepared for photocatalytic… Show more

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