Construction of three novel Co/Zn/Cd(II) coordination polymers based on the same ligands: Different spatial structures, electrocatalysis and photoluminescence properties

Gao, Jia-Hao; Huang, Pei-Pei; Liu, Jie; Zheng, Nan; Wang, Dong; Yue, Si-Yu; Liu, Er-Nu; Liu, Quan; Liu, Bo; Lu, Jiu-Fu

doi:10.1016/j.arabjc.2023.105314

Arabian Journal of Chemistry

2023

DOI: 10.1016/j.arabjc.2023.105314

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Construction of three novel Co/Zn/Cd(II) coordination polymers based on the same ligands: Different spatial structures, electrocatalysis and photoluminescence properties

Jia-Hao Gao,

Pei-Pei Huang,

Jie Liu

et al.

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Cited by 7 publications

References 36 publications

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Single‐crystal‐to‐single‐crystal transformation of a two‐dimensional noninterpenetrated layer to a microporous three‐dimensional fourfold interpenetrated MOF triggered by DMF

Huang,

Wu,

Tuo

et al. 2024

Applied Organom Chemis

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We have demonstrated a single‐crystal‐to‐single‐crystal (SCSC) transformation from a two‐dimensional noninterpenetrated layer to a microporous three‐dimensional fourfold interpenetrated MOF. The centrosymmetric [Co2(μ2‐OH)(EIBA)3]n (SNUT‐25) transforms into a microporous [Co(EIBA)2]n (SNUT‐26), which is triggered by the reaction time with DMF that acts as a structure‐directing agent (HEIBA = 4‐(2‐ethyl‐1H‐imidazol‐1‐yl)benzoic acid; DMF = N,N′‐dimethylformamide). Despite the distinct structure and coordination arrangements of SNUT‐25 in contrast to SNUT‐26, both Co‐MOFs were synthesized using the same ligand. Fascinatingly, upon introducing a specific quantity of DMF combined with a negligible proportion of nitric acid, SNUT‐25 will progressively and completely transform into SNUT‐26. Under the synergistic induction of solvent molecules and temperature, SNUT‐25 changed from the original two‐dimensional layered structure to the three‐dimensional pore structure of SNUT‐26. In addition, SNUT‐25 and SNUT‐26 are efficient photocatalysts for the degradation of organic dye methyl blue (MB) under visible light irradiation. Surprisingly, the degradation rates of both SNUT‐25 and SNUT‐26 can reach over 96%. In addition, SNUT‐25 and SNUT‐26 also exhibited high electrocatalytic oxygen evolution reaction.

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Single‐crystal‐to‐single‐crystal transformation of a two‐dimensional noninterpenetrated layer to a microporous three‐dimensional fourfold interpenetrated MOF triggered by DMF

Huang,

Wu,

Tuo

et al. 2024

Applied Organom Chemis

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A new 3D Cd-MOF with 2fold interpenetrated as “turn-on/turn-off” fluorescent sensor for selective and sensitive detection of Cu2+, Al3+ and Fe3+ ions

Gao,

Huang,

Zhang

et al. 2024

Journal of Molecular Structure

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Supramolecular complexes of Co(II), Zn(II) and Mn(II) based on a pyridazine dicarboxylic derivative: Synthesis, crystal structures and properties

Huang,

Wu,

Tuo

et al. 2024

Journal of Molecular Structure

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Construction of three novel Co/Zn/Cd(II) coordination polymers based on the same ligands: Different spatial structures, electrocatalysis and photoluminescence properties

Cited by 7 publications

References 36 publications

Single‐crystal‐to‐single‐crystal transformation of a two‐dimensional noninterpenetrated layer to a microporous three‐dimensional fourfold interpenetrated MOF triggered by DMF

Single‐crystal‐to‐single‐crystal transformation of a two‐dimensional noninterpenetrated layer to a microporous three‐dimensional fourfold interpenetrated MOF triggered by DMF

A new 3D Cd-MOF with 2fold interpenetrated as “turn-on/turn-off” fluorescent sensor for selective and sensitive detection of Cu2+, Al3+ and Fe3+ ions

Supramolecular complexes of Co(II), Zn(II) and Mn(II) based on a pyridazine dicarboxylic derivative: Synthesis, crystal structures and properties

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