2023
DOI: 10.1002/ange.202314523
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Controlling Electron Delocalization in Vanadium‐Based Hybrid Bronzes through Molecular Templation

Suchen Wan,
Nicole Musielak,
Allen G. Oliver
et al.

Abstract: We show that the conductivity of hybrid vanadium bronzes—mixed‐valence organic‐inorganic vanadium oxides—can be tuned over six orders of magnitude through judicious choice of molecular component. By systematically varying the steric profile, charge density, and propensity to hydrogen bond across a series of eight diammonium‐based molecules, we engender multiple distinct motifs of V–O connectivity within the two‐dimensional vanadium oxide layers of a family of bulk crystalline hybrid materials. A combination of… Show more

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