Controlling Resonance Fluorescence Spectra and Photon Statistics in a Driven V-Type Quantum Emitter—Metal Nanoparticle Coupled Structure

Abstract

We study the resonant fluorescence emission spectrum and the intensity-intensity correlations of the emitted fluorescent field by a V-type quantum emitter (QE) which is located near a metal nanosphere. For the description of the studied phenomena, we use the density matrix equations methodology combined with electromagnetic calculations and obtain results for the profile of the resonant fluorescence spectrum and the second-order correlation functions associated with the fluorescent photons. The decay rates and the coupling term exhibit a strong dependence on the distance that separates the QE from the metal nanoparticle. This distance also influences the resonance fluorescence of the V-type QE. We find that, in the general case, the resonant fluorescence spectrum is composed of five Lorentzian-type peaks, for high interparticle distances, while, when the QE is located very close to the surface of the nanosphere, the central resonance becomes dominant, and a single-peaked spectral profile appears. The two-time correlation functions of the fluorescent photons evolve in an oscillatory manner around unity, for non-zero time delay, with a period that decreases with the increase of the field intensity. In the strong driving field regime, the antibunching to bunching crossing time does not depend on the interparticle distance, contrary to the results found in the weak driving field regime. We also find that, for a weak laser field and under specific conditions, the second-order correlation functions constantly remain in the antibunching region.

Modification of the Emission Spectrum of a Quantum Emitter in the Vicinity of Bismuth Chalcogenide Microparticles

“…This occurs when there is a substantial difference in decay rates between orthogonal dipole moments, resulting in a noticeable degree of QI [27]. This phenomenon in a quantum emitter could result in exciting phenomena in quantum optics and coherent nonlinear optics, including coherent population trapping [28][29][30][31][32], a large degree of entanglement [33][34][35], amplification without inversion [36,37], controllable spontaneous emission or resonance fluorescence spectra [26,[38][39][40], optical transparency accompanied with slow light [41][42][43], strengthened Kerr nonlinearity [44][45][46][47][48], and distinct non-Markovian dynamics [49].…”