2015
DOI: 10.1088/1367-2630/17/12/123026
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Controlling ultrafast currents by the nonlinear photogalvanic effect

Abstract: We investigate the effect of broken inversion symmetry on the generation and control of ultrafast currents in a transparent dielectric (SiO 2 ) by strong femtosecond optical laser pulses. Ab initio simulations based on time-dependent density functional theory predict ultrafast direct currents that can be viewed as a nonlinear photogalvanic effect. Most surprisingly, the direction of the current undergoes a sudden reversal above a critical threshold value of laser intensity of about I 3 10 c 13Ẃ cm −2 . We trac… Show more

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Cited by 26 publications
(19 citation statements)
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“…This application exemplifies time-resolved measurements with a subfemtosecond sampling signal, which is referred to as attosecond metrology (Hentschel et al, 2001;Krausz and Stockman, 2014). Employing the waveform control to investigate and possibly extend the frontiers of signal processing in electronics is another intriguing idea Lee et al, 2016;Wachter et al, 2015). Even from a purely academic perspective, studying the nonequilibrium electron dynamics on the femtosecond scale present numerous research opportunities, one of which is the transition from ballistic to dissipative electron transport in a pump-probe setting (Wachter et al, 2014).…”
Section: B Light-waveform Control Of Electric Currentmentioning
confidence: 99%
“…This application exemplifies time-resolved measurements with a subfemtosecond sampling signal, which is referred to as attosecond metrology (Hentschel et al, 2001;Krausz and Stockman, 2014). Employing the waveform control to investigate and possibly extend the frontiers of signal processing in electronics is another intriguing idea Lee et al, 2016;Wachter et al, 2015). Even from a purely academic perspective, studying the nonequilibrium electron dynamics on the femtosecond scale present numerous research opportunities, one of which is the transition from ballistic to dissipative electron transport in a pump-probe setting (Wachter et al, 2014).…”
Section: B Light-waveform Control Of Electric Currentmentioning
confidence: 99%
“…We use TDDFT in a real-space real-time implementation [36,37] to simulate the electronic dynamics driven by the strong IR field F (t) employing the adiabatic localdensity approximation (LDA). Alternatively, we implement the SBEs by propagating the elements of the density matrix ρ k mn ,…”
mentioning
confidence: 99%
“…is the vector potential of the driving laser, and C is an adjustable parameter. As already demonstrated [26], the charge can be obtained by and his co-workers also found a sudden reversal of the directional currents above critical threshold intensity in their simulation based on time-dependent density functional theory [27]. In 6 their case, CEP effect was removed by applying a longer laser pulse.…”
Section: Results and Disscussionmentioning
confidence: 65%