2019
DOI: 10.1002/smll.201902779
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Coordination‐Driven Hierarchical Assembly of Hybrid Nanostructures Based on 2D Materials

Abstract: nanobelts), 2D materials exhibit exceptional physical properties including large theoretical surface area, tunable electronic properties, high optical transparency, and excellent mechanical properties. [2] However, the strong re-stacking tendency of 2D materials caused by van der Waals interaction may result in serious loss of surface area, which inevitably weakens their unique properties. Besides, 2D materials always show intrinsic deficiencies for specific applications, despite the merits mentioned above. As… Show more

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Cited by 14 publications
(11 citation statements)
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References 225 publications
(396 reference statements)
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“…Surfactant dispersions used to confine LC samples can be used to encode spatial information leading to specific arrangements [66,67]. Structured colloidal assemblies via topological defects can impart screw/twist symmetry in colloidal assemblies [193][194][195][196], thereby facilitating the production of chiral materials. Switching dynamics controllable through external fields (i.e., electric, magnetic, photonic, etc.)…”
Section: Dimensionality and Confined Liquid Crystal Samplesmentioning
confidence: 99%
“…Surfactant dispersions used to confine LC samples can be used to encode spatial information leading to specific arrangements [66,67]. Structured colloidal assemblies via topological defects can impart screw/twist symmetry in colloidal assemblies [193][194][195][196], thereby facilitating the production of chiral materials. Switching dynamics controllable through external fields (i.e., electric, magnetic, photonic, etc.)…”
Section: Dimensionality and Confined Liquid Crystal Samplesmentioning
confidence: 99%
“…Gogotsi manufactured flexible MXene/rGO films through electrostatic self-assembly, and rGO sheets embedded between MXene layers effectively prevent the self-stacking of MXene and rGO sheets. These above results indicate that the self-stacking of 2D materials can be alleviated by electrostatic self-assembly and hydrogen bond interaction. , However, it is still a considerable challenge that effectively addresses structural instability caused by the volume expansion of 2D materials during ion insertion/extraction processes. Compared with electrostatic self-assembly and hydrogen bonding, the covalent bonding combination is a strong interaction in constructing robust 2D layered nanocomposites, which can provide a more stable structure to facilitate fast Li + ion transfer rates. …”
Section: Introductionmentioning
confidence: 99%
“…3−6 However, despite tremendous progress, mimicking the intrinsic features of natural structural hierarchy through nanostructure assembly is still challenging. 7,8 In particular, the natural hierarchical organisms are generated through growth evolution, which can adapt to their growth environments, allowing the formation of entities with diversified shapes across a wide length scale. 9,10 In contrast, artificially assembled hierarchical materials are normally restricted to regular shapes (such as rods and spheres) and specific sizes.…”
Section: ■ Introductionmentioning
confidence: 99%
“…The assembly of nano building blocks into three-dimensional hierarchical architectures is enormously appealing from the perspectives of both fundamental research and practical applications due to the sophisticated assembly process and the extraordinary properties of the resultant materials. , As powerful sources of inspiration, natural organisms possessing the advantages of multilevel hierarchy, morphological diversity, and large length scale have been extensively pursued for hierarchical architecture assembly. However, despite tremendous progress, mimicking the intrinsic features of natural structural hierarchy through nanostructure assembly is still challenging. , In particular, the natural hierarchical organisms are generated through growth evolution, which can adapt to their growth environments, allowing the formation of entities with diversified shapes across a wide length scale. , In contrast, artificially assembled hierarchical materials are normally restricted to regular shapes (such as rods and spheres) and specific sizes . This is primarily attributed to the inherent requirements of traditional assembly, that is, straightforward assembly of nanostructures for the thermodynamic equilibrium of the system, which confines the morphology of the resulting assemblage to a regular shape and specific size to achieve minimum surface energy. Hence, to address this issue, it is imperative to explore a novel strategy distinct from traditional assembly to create hierarchical materials with greater diversity in terms of 3D shapes and dimensions.…”
Section: Introductionmentioning
confidence: 99%