The magnetized zeolite with an optimized conversion rate of 53% can be readily synthesized from industrial anthracite using a water-based method. The highly porous structure of ferromagnetism zeolite demonstrates robust magnetic properties with a magnetite content of 12–15%, satisfying adsorbent separation and recycling through magnetic cylinder rotating and vibrating separation. A cesium adsorption and removal efficiency as high as 99.92% with a corresponding adsorbent recovery ratio of up to 96.36% can be achieved for the simulated cesium-contaminated soil with a water content of 20% and a cesium content of 1% with an adsorbent-to-contaminated soil ratio of 1:2. Adsorption and magnetic separation technology with magnetized zeolite synthesized from anthracite exhibited a high cesium removal rate and zeolite recovery ratio, demonstrating promising application potential in treating radioactive waste soils and robust and economically viable engineering feasibility.