Seismic tomography models have discerned the presence of two mantle structures close to the core-mantle interface characterized by low seismic velocities. These large low-shear velocity provinces (LLSVPs) sit beneath Africa and the Pacific plate and exhibit a shear velocity anomaly of δlnV s ≈ −2%. Spatially, they are both voluminous and broad (Cottaar & Lekić, 2016), with seismic tomography models showing high power in spherical harmonic degree 2 and to a lesser extent degree 3 structures (Koelemeijer et al., 2016;Ritsema et al., 2011) in the lower mantle. These structures exist within and above the D" layer and may extend >1,000 km into the mantle from the core-mantle boundary (CMB) (He & Wen, 2009;Lekic et al., 2012), with the African LLSVP being significantly taller than the Pacific LLSVP (Ni et al., 2002;Yuan & Li, 2022). Mantle plumes are claimed to cluster around their edges (Thorne et al., 2004) potentially entraining material to be sampled by melting beneath ocean islands. Despite the morphology of LLSVPs being well constrained, increasingly accurate measurements of their material properties and possible direct links to the surface via plumes, their origin and composition remain a matter of debate. This is because the very characteristics that define LLSVPs have a non-unique source; the velocity anomaly may originate thermally, chemically, or thermo-chemically. Consequently there are competing theories over the nature of LLSVPs, are they of a predominantly thermal origin (D. R. Davies et al., 2015;