Coupling electrochemical CO<sub>2</sub> reduction with value-added anodic oxidation reactions: progress and challenges

Li, Yu; Lu, Tong-Bu

doi:10.1039/d3qm00625e

Mater. Chem. Front.

2024

DOI: 10.1039/d3qm00625e

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Coupling electrochemical CO₂ reduction with value-added anodic oxidation reactions: progress and challenges

Yu Li,

Tong-Bu Lu

Abstract: Converting CO2 into chemicals using renewable electricity provides a promising avenue to realize carbon neutrality. Substituting the anodic oxygen evolution reaction by thermodynamically more favourable oxidation reactions with value-added products...

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Atomically Precise Cu Nanoclusters: Recent Advances, Challenges, and Perspectives in Synthesis and Catalytic Applications

Chen,

Guo,

Qin

et al. 2024

Nano-Micro Lett.

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Atomically precise metal nanoclusters are an emerging type of nanomaterial which has diverse interfacial metal–ligand coordination motifs that can significantly affect their physicochemical properties and functionalities. Among that, Cu nanoclusters have been gaining continuous increasing research attentions, thanks to the low cost, diversified structures, and superior catalytic performance for various reactions. In this review, we first summarize the recent progress regarding the synthetic methods of atomically precise Cu nanoclusters and the coordination modes between Cu and several typical ligands and then discuss the catalytic applications of these Cu nanoclusters with some explicit examples to explain the atomical-level structure–performance relationship. Finally, the current challenges and future research perspectives with some critical thoughts are elaborated. We hope this review can not only provide a whole picture of the current advances regarding the synthesis and catalytic applications of atomically precise Cu nanoclusters, but also points out some future research visions in this rapidly booming field.

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Atomically Precise Cu Nanoclusters: Recent Advances, Challenges, and Perspectives in Synthesis and Catalytic Applications

Chen,

Guo,

Qin

et al. 2024

Nano-Micro Lett.

View full text Add to dashboard Cite

show abstract

Electrochemical CO₂ Conversion Commercialization Pathways: A Concise Review on Experimental Frontiers and Technoeconomic Analysis

Kumar,

Muchharla,

Dikshit

et al. 2024

Environ. Sci. Technol. Lett.

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Technoeconomic analysis (TEA) studies are vital for formulating guidelines that drive the commercialization of electrochemical CO 2 reduction (eCO 2 R) technologies. In this review, we first discuss the progress in the field of eCO 2 R processes by providing current state-of-the-art metrices (e.g., faradic efficiency, current density) based on the recent heterogeneous catalysts' discovery, electrolytes, electrolyzers configuration, and electrolysis process designs. Next, we assessed the TEA studies for a wide range of eCO 2 R final products, different modes of eCO 2 R systems/processes, and discussed their relative competitiveness with relevant commercial products. Finally, we discuss challenges and future directions essential for eCO 2 R commercialization by linking suggestions from TEA studies. We believe that this review will catalyze innovation in formulating advanced eCO 2 R strategies to meet the TEA benchmarks for the conversion of CO 2 into valuable chemicals at the industrial scale.

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Coupling electrochemical CO₂ reduction with value-added anodic oxidation reactions: progress and challenges

Abstract: Converting CO2 into chemicals using renewable electricity provides a promising avenue to realize carbon neutrality. Substituting the anodic oxygen evolution reaction by thermodynamically more favourable oxidation reactions with value-added products...

Cited by 2 publications

References 80 publications

Atomically Precise Cu Nanoclusters: Recent Advances, Challenges, and Perspectives in Synthesis and Catalytic Applications

Atomically Precise Cu Nanoclusters: Recent Advances, Challenges, and Perspectives in Synthesis and Catalytic Applications

Electrochemical CO₂ Conversion Commercialization Pathways: A Concise Review on Experimental Frontiers and Technoeconomic Analysis

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Coupling electrochemical CO2 reduction with value-added anodic oxidation reactions: progress and challenges

Abstract: Converting CO2 into chemicals using renewable electricity provides a promising avenue to realize carbon neutrality. Substituting the anodic oxygen evolution reaction by thermodynamically more favourable oxidation reactions with value-added products...

Cited by 2 publications

References 80 publications

Atomically Precise Cu Nanoclusters: Recent Advances, Challenges, and Perspectives in Synthesis and Catalytic Applications

Atomically Precise Cu Nanoclusters: Recent Advances, Challenges, and Perspectives in Synthesis and Catalytic Applications

Electrochemical CO2 Conversion Commercialization Pathways: A Concise Review on Experimental Frontiers and Technoeconomic Analysis

Contact Info

Product

Resources

About

Coupling electrochemical CO₂ reduction with value-added anodic oxidation reactions: progress and challenges

Electrochemical CO₂ Conversion Commercialization Pathways: A Concise Review on Experimental Frontiers and Technoeconomic Analysis