Decoupling between propagating acoustic waves and two-level systems in hydrogenated amorphous silicon

Abstract

Specific heat measurements of hydrogenated amorphous silicon prepared by hot-wire chemical vapor deposition show a large density of two-level systems at low temperature. Annealing at 200• C, well below the growth temperature, does not significantly affect the already-low internal friction or the sound velocity, but irreversibly reduces the non-Debye specific heat by an order of magnitude at 2 K, indicating a large reduction of the density of two-level systems. Comparison of the specific heat to the internal friction suggests that the two-level systems are uncharacteristically decoupled from acoustic waves, both before and after annealing. Analysis yields an anomalously low value of the coupling constant, which increases upon annealing but still remains anomalously low. The results suggest that the coupling constant value is lowered by the presence of hydrogen.

Transport and relaxation of current-generated nonequilibrium phonons from nonlocal electronic measurements

“…Such dynamics may be related to the bosonic peak ubiquitous in the spectra of amorphous materials [37][38][39] and to the problem of phonon glass [40,41], and may be associated with quasilocalized nonlinear defect states such as bistable atomic configurations [top inset in Fig. 4(a)], as well as interstitial impurities and incoherent interfaces [42,43].…”