Aerosols modulate Earth's energy balance both directly and indirectly. Directly they scatter or absorb solar radiation, and indirectly they alter cloud micro-and macro-physical properties by serving as cloud ice and condensation nuclei (Boucher et al., 2013;Y. Wang et al., 2014). The effective radiative forcing (ERF, defined as Earth's energy imbalance to a radiative perturbation) (Forster et al., 2016;Myhre et al., 2013) from aerosol-radiation-interaction (ERFari) and aerosol-cloud interaction (ERFaci) due to changes in aerosol concentrations in the industrial era (present-day, PD) relative to preindustrial (PI) levels has been quantified by global climate models (GCMs). In the fifth phase of the Coupled Model Intercomparison Project (CMIP5), the total (shortwave + longwave) ERF due to anthropogenic aerosols (ERFari + aci) was estimated to be −1.17 ± 0.30 W/m 2 , with ERFari of −0.25 ± 0.22 W/m 2 and ERFaci of −0.92 ± 0.34 W/m 2 , respectively (Zelinka et al., 2014). Its updated value from CMIP6 models is −1.04 ± 0.20 W/m 2 , with −0.23 ± 0.19 W/m 2 from ERFari and −0.81 ± 0.30 W/m 2 from ERFaci (Smith et al., 2020). Observationally, Chung et al. (2005) estimated ERFari to be −0.35 W m −2 with a range of −0.6 to −0.1 W m −2 from satellite and ground-based observations. Using satellite-based estimation, Jia