2024
DOI: 10.1021/acsaenm.3c00747
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Defect Tailoring in the Metal–Organic Framework Cu (BDC-NH2) for the High-Efficiency Photocatalytic Reduction of Cr(VI)

Liyue Tao,
Junjie Ren,
Zhaoyue Luo
et al.

Abstract: Mixed-linker metal−organic frameworks of Cu (BDC-NH 2 ) have been fabricated in which the 2-aminoterephthalic acid (BDC-NH 2 ) linker has been partially replaced by 3,5-pyridinedicarboxylic acid (PYDC) without obviously changing the crystal structure. The pyridine unit, as a defect site in the local coordination environment of the dimitic copper units, can alter the electronic structure. The experimental results of the photocatalytic reduction of Cr(VI) reveal that defect engineering can effectively modify the… Show more

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