2007
DOI: 10.1016/j.catcom.2006.09.003
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Dehydration of 1,4-butanediol over lanthanide oxides

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Cited by 48 publications
(19 citation statements)
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“…In our previous work, we have studied the vapor-phase dehydration of 1,3-butanediol [13][14][15][16][17][18], 1,4-butanediol [19][20][21][22][23], and 1,5-pentanediol [24,25]. Well-crystallized oxide surface such as CeO 2 (111) is effective in the selective formation of unsaturated alcohol in the dehydration [14].…”
Section: Introductionmentioning
confidence: 99%
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“…In our previous work, we have studied the vapor-phase dehydration of 1,3-butanediol [13][14][15][16][17][18], 1,4-butanediol [19][20][21][22][23], and 1,5-pentanediol [24,25]. Well-crystallized oxide surface such as CeO 2 (111) is effective in the selective formation of unsaturated alcohol in the dehydration [14].…”
Section: Introductionmentioning
confidence: 99%
“…A theoretical study of the adsorption of 1,3-butanediol suggests that the dehydration of 1,3-butanediol proceeds at the oxygen-defect sites of the CeO 2 (111) surface through the redox cycle between Ce 4+ and Ce 3+ [16][17][18]. In the dehydration of 1,4-butanediol, preferential formation of 3-buten-1-ol was observed over CeO 2 [19], ZrO 2 [20], Yb 2 O 3 [21], and Er 2 O 3 [22]. It is also known that Er 2 O 3 , Tm 2 O 3 , Yb 2 O 3 , and Lu 2 O 3 also work well for the formation of 3-buten-1-ol from 1,4-butanediol at 325°C when they are supported on ZrO 2 [23].…”
Section: Introductionmentioning
confidence: 99%
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“…In addition, BDO is selectively dehydrated into THF over strong acid catalysts. [25][26][27][28][29] The inuence of supported copper catalysts on dehydrogenation of BDO to GBL has been examined. 1,4,24,30 Since, the dehydrogenation of BDO to GBL is favourable over acid supported catalysts, it has been conducted over acidic supported catalysts such as Cu/Cr/Mn, Cu/Cr/Zn and Cu/Zn/Al.…”
Section: Catalytic Activitymentioning
confidence: 99%
“…At the same time tetrahydrofuran (THF) can be synthesized from BDO by employing acid catalyse systems via dehydration. [25][26][27][28][29] The enormous importance of these chemicals, due to derive from biomass, BDO conversion has received great attention.…”
Section: Introductionmentioning
confidence: 99%