Marble and limestone surfaces were exposed to atmospheric conditions at four eastern U.S. sites and were monitored for changes in surface chemistry, surface roughness/recession, and weight. The effect of acid deposition, to which calcareous materials are especially sensitive, was of particular interest. Results are described for the first year of testing, and aspects of a preliminary equation to relate damage to environmental factors are discussed.Thus far, findings support that acid deposition substantially damages marble and limestone surfaces.Improvements in methods to reduce uncertainties in the quantitative contributions of important chemical species are outlined for the ongoing effort.