2023
DOI: 10.1002/hlca.202200191
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Destabilizing Predictive Copper‐Catalyzed Click Reactions by Remote Interactions with a Zinc‐Porphyrin Backbone

Abstract: In order to obtain new supramolecular ligands that build up around a zinc‐porphyrin scaffold, we envisioned to access sulfonyl triazole intermediates by well‐known copper‐catalyzed click reactions. Unexpectedly, these triazole intermediates do not form due to the presence of the zinc‐porphyrin moiety at close proximity of the active copper species. Indeed, the copper catalyst undergoes a different chemo‐selective reaction pathway reacting with traces of alcohols or water from the media that behave as effective… Show more

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Cited by 2 publications
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