Strongly correlated quantum systems can exhibit exotic behavior controlled by topology. We predict that the ν = 1/2 fractional Chern insulator arises naturally in a two-dimensional array of driven, dipolar-interacting spins. As a specific implementation, we analyze how to prepare and detect synthetic gauge potentials for the rotational excitations of ultra-cold polar molecules trapped in a deep optical lattice. While the orbital motion of the molecules is pinned, at finite densities, the rotational excitations form a fractional Chern insulator. We present a detailed experimental blueprint for 40 K 87 Rb, and demonstrate that the energetics are consistent with near-term capabilities. Prospects for the realization of such phases in solid-state dipolar systems are discussed as are their possible applications.The quest to realize novel forms of topological quantum matter has recently been galvanized by the theoretical prediction and subsequent experimental observation of topological insulators [1, 2]. Such materials harbor an insulating bulk, but owing to nontrivial bulk topology, they are also characterized by robust conducting surface states. Recent theoretical work has shown that combining single particle topological bands with strong interactions can yield so-called fractional Chern insulating (FCI) phases [3][4][5][6][7][8]. Particles injected into these exotic states of matter fractionalize into multiple independently propagating pieces, each of which carries a fraction of the original particle's quantum numbers. Unlike traditional bosons or fermions, these anyonic excitations accumulate a nontrivial phase under exchange.While similar effects underpin the fractional quantum Hall effect observed in continuum two dimensional electron gases [10], fractional Chern insulators, by contrast, are lattice dominated. They have an extremely high density of correlated particles whose collective excitations can transform non-trivially under lattice symmetries [8, 9]. In this paper, we predict the existence of a FCI state in dipolar interacting spin systems (see Fig. 1). This state exhibits fractionalization of the underlying spins into quasiparticle pairs with semionic statistics [11]. The predicted FCI state may also be viewed as a gapped chiral spin liquid [11,12], a state which has never been observed in nature. Such a state cannot be realized in conventional electron gases.Several recent studies have conjectured the existence of fractionalized topological phases in idealized lattice models that require sensitively tuned long-range hopping and interactions [5][6][7][13][14][15]. Broadly speaking, two single-particle microscopic ingredients are required, both of which find close analogy in the physics of the electronic Hall effect. First, just as electrons in a Landau level have no dispersion, the dispersion of the lattice band-structure must be quenched relative to the energy scale of interactions. This enables interactions between particles to dominate over the kinetics of their environment [13][14][15]. Second, the fl...