The erodibility and erosion resistance of Quaternary sediments play a pivotal role in both the hydrologic and erosion processes of soil cut slopes. To investigate the runoff and sediment yield of soil cut slopes along the Pai-Mo road, we performed indoor simulated rainfall experiments under a 50° steep slope and high rainfall intensity (120 mm/h), based on the area’s climatic characteristics and Quaternary sediment properties. The experiments included various rock fragment contents (30%, 40%, and 50%), different levels of rock fragment roundness (i.e., rounded gravel, angular gravel), and varying soil cohesion. The results indicated that the average infiltration rate of the uncemented rounded gravel soil slope (URGSS) was higher than that of the uncemented angular gravel soil slope (UAGSS), resulting in less runoff and a delayed initial runoff time. The runoff shear stress, runoff power, drag coefficient, and Reynolds number of the URGSS were smaller than those of the UAGSS. In contrast, the Froude number and flow velocity of the URGSS were larger, resulting in a stronger runoff erosion capacity. The sediment yield of the URGSS was approximately two times that of the UAGSS, and the cumulative sediment yield was about 20% higher. The cemented angular gravel soil slope (CAGSS) had a larger runoff rate, runoff shear stress, runoff power, and flow velocity than those of the UAGSS, leading to less sediment yield. Overall, a more rounded shape and a larger radius of curvature of the spherical particles resulted in stronger erosion, due to local turbulence. Therefore, the rill density and cumulative sediment yield of the steep alluvial cut slope were greater than that of the steep colluvial cut slope under heavy rainfall. Moreover, due to its strong cohesion, only raindrop splash erosion and inter-rill erosion occurred on the steep moraine cut slopes under heavy rainfall.