This paper experimentally examines the influence of hybrid excitation on the performance of vibrational piezoelectric energy harvesting systems on a bluff body with a variable cross section along its generatrix. A combination of vibrational excitation from a shaker and airflow is considered the source from which energy is harvested. Varied excitation frequencies and airflow velocities across five different masses were considered, each defining the natural frequency of the system. The system’s performance in hybrid excitation, enhancements in energy harvesting, and challenges with these was observed, helping to determine optimal operating conditions to function effectively in ambient environments. The tests identified the conditions and ranges within which maximized harvesting responses were observed. Next, computational fluid dynamic (CFD) simulations were carried out to understand the impact of circular and square cross sections controlling the nature of the airflow and representative of the wide range of cross sections that may be utilized for such purposes. The analyses helped contextualize the opportunities and limitations of the use of such cross sections and helped in understanding if a transition from one cross section to another can lead to an assimilation of the advantages observed in using each cross section independently.