“…As can be seen from Figure 4 b, the dielectric constant of the composites increased with the increase in F-graphene content, and the dielectric constant of pure epoxy resin was 4.86 at 1 kHz frequency, while that of F-graphene/epoxy composites reached 8.23 at an F-graphene loading of 1.0 wt.%, which was about 1.69 times that of pure epoxy. This can be attributed to the interfacial polarization effect introduced by F-graphene nanofiller doping, i.e., because of the significant difference in dielectric properties (e.g., polarity and dielectric constant) between inorganic F-graphene and organic epoxy resin matrix, a high-intensity local electric field is formed at the interface of the two phases, and the free electrons generated within the composite dielectric under the applied electric field are captured at the interface of the two phases, i.e., the charge accumulates in the interfacial region with high field strength, which leads to the increase in space charge within the composites and thus the elevation of the dielectric constant [ 55 , 56 , 57 , 58 , 59 ]. In this study, the interfacial polarization effect can be explained more intuitively by the micro-capacitance model [ 60 , 61 ].…”