“…Yet, stratospheric solar 15 geoengineering (SSG) scenarios differ from volcanic aerosol injections in that with SSG sulfur will presumably be injected into aircraft plumes, producing high local concentrations and strong gradients, and because emissions will be continuous in time, factors which will yield different microphysical behaviour (Heckendorn et al, 2009). Studies of SSG by injection of gas phase SO 2 have found limitations including: (1) reduced efficacy at higher loading due to unfavorable aerosol size distributions with possible limitations on achievable radiative forcing (Heckendorn et al, 20 2009;English et al, 2012;Niemeier and Timmreck, 2015), (2) depletion of stratospheric ozone (Tilmes et al 2009;Pitari et al 2014), (3) stratospheric heating which also perturbs stratospheric circulation and water vapor (Ferraro et al, 2011;Aquila et al, 2014;Richter et al, 2017;Niemeier amd Schmidt, 2017;Franke et al, 2021), (4) enhanced diffuse light at the Earth' surface (Kravitz et al, 2012), and (5) impacts on upper tropospheric ice clouds (Kuebbeler et al, 2012;Visioni et al, 2018a). These limitations might be addressed through use of various solid aerosol particles for SSG (e.g.…”