“…As an important class of optoelectronic devices, photodetectors are applied in many fields, including optical communication, image sensing, and chemical/biological detection. − Recently, photodetectors comprising graphene films and graphene derivatives have attracted tremendous notice because of their unique chemical/physical properties. The extremely high carrier mobility of graphene films enables ultrafast conversion from photons to electrical signals to facilitate high-speed photodetection. , Additionally, the optical/electrical properties of graphene films, especially the band alignments, carrier densities, and polarities, can be tuned precisely by adjusting chemical or electrostatic doping, consequently providing more flexibility in optimizing the performance of photodetectors. , However, the low light absorption rate (2.3% for monolayer graphene films) and short exciton lifetime characteristics of pristine graphene hamper its practical application. ,− To obtain higher properties of graphene film-based photodetectors, some techniques such as graphene film functional modification, , assembly of heterojunctions, , and changing the morphology of graphene films , have been proposed and these techniques have made great progress.…”