We investigate two measures of quantum correlations and entanglement, namely the violation of the Bell-Mermin-Klyshko (BMK) inequalities and the quantum discord, for Dirac fermions in the cosmological de Sitter background of dimension four. The BMK violation is focused on the vacuum for two-and four-mode squeezed states and the maximum violation is demonstrated. For the quantum discord, we investigate a maximally entangled in-vacuum state. Qualitative similarities as well as differences of our results with that of different coordinations of de Sitter in the context of scalar and fermionic field theory are discussed.