Direct Synthesis of Organic Carbonates from CO<sub>2</sub>and Alcohols Using Heterogeneous Oxide Catalysts

Nakagawa, Yoshinao; Honda, Masayoshi; Tomishige, Keiichi

doi:10.1002/9781118831922.ch5

Green Carbon Dioxide 2014

DOI: 10.1002/9781118831922.ch5

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Direct Synthesis of Organic Carbonates from CO₂and Alcohols Using Heterogeneous Oxide Catalysts

Yoshinao Nakagawa

Masayoshi Honda²,

Keiichi Tomishige

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2024

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Cited by 2 publications

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Sustainable Valorization of CO2 through Nuclear Power-to-X Pathways

Ramirez-Corredores

2024

Energies

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Some of the issues concerning energy security and climate change can be addressed by employing nuclear power (NP) to supply the energy required for the conversion of carbon dioxide (CO2) into chemicals, products, and materials. Nuclear energy represents a neutral carbon source that can be generated sustainably, reliably, and consistently. Nuclear power plants (NPPs) could supply energy in the form of heat, electricity, and ionizing radiation to drive CO2 chemical reactions underpinning NP-to-X type of pathways. CO2 conversion processes are either commercially available or emerging technologies at different developmental maturity stages. This work reviews the published literature (articles and patents) that reports R&D results and the understanding and development of chemical reactions and processes, as well as the efforts in integrating NPPs and chemical processes (CPs). As will be made evident, a new industrial era for the manufacturing of decarbonized chemicals, products, and materials will be possible by developing and implementing new (more energy- and carbon-efficient) processes responding to the NP-to-X pathways. This new decarbonizing platform not only contributes to achieving net zero goals but also broadens the NPP product beyond electricity.

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Sustainable Valorization of CO2 through Nuclear Power-to-X Pathways

Ramirez-Corredores

2024

Energies

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A Carbon Dioxide Refinery: The Core of a Sustainable Carbon-based Circular Economy

Ramirez-Corredores

2024

Highlights Sustain.

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The atmospheric carbon dioxide (CO2) accumulation (2–2.5 ppmv/year) is the result of the enormous gap between its emissions (37 Gton/year) and its capture, storage, and utilization (<500 Mton/year). Climate has been dramatically affected due to the failure of natural sinks, in working effectively. To address this Gton-scale gap, numerous uses and applications are needed particularly, those consuming vast volumes of this compound and/or rendering longevous products or long lifecycle services. Thus, carbon utilization (CU) can be seen as the step to close the carbon cycle. Among CU, R&D on CO2 chemical conversion has proposed a variety of processes, with different degrees of developmental maturity. These chemical process technologies could be efficiently and effectively integrated into refineries to upgrade emitted CO2. A technology pipeline consisting of a database of these processes and the technology market status should be defined based on published scientific results and patents. Then, an innovative top-down methodology is proposed to eco-design configurations of that refinery, to warrant a sustainable carbon cycle (in terms of energy, environment, and economy) and to change the ways of producing fuels, chemicals, and materials. Additionally, the proposed methodology could be used to identify research and development gaps and needs, for orienting science and technology investments and measures. Hopefully, sustainable CO2 refineries will be implemented to close the carbon cycle of a circular C-based economy and underpin a decarbonized chemical industry.

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Direct Synthesis of Organic Carbonates from CO₂and Alcohols Using Heterogeneous Oxide Catalysts

Cited by 2 publications

References 64 publications

Sustainable Valorization of CO2 through Nuclear Power-to-X Pathways

Sustainable Valorization of CO2 through Nuclear Power-to-X Pathways

A Carbon Dioxide Refinery: The Core of a Sustainable Carbon-based Circular Economy

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Direct Synthesis of Organic Carbonates from CO2and Alcohols Using Heterogeneous Oxide Catalysts

Cited by 2 publications

References 64 publications

Sustainable Valorization of CO2 through Nuclear Power-to-X Pathways

Sustainable Valorization of CO2 through Nuclear Power-to-X Pathways

A Carbon Dioxide Refinery: The Core of a Sustainable Carbon-based Circular Economy

Contact Info

Product

Resources

About

Direct Synthesis of Organic Carbonates from CO₂and Alcohols Using Heterogeneous Oxide Catalysts